Modeling of NH 3-NO-SCR reaction over CuO/γ-Al 2O 3 catalyst in a bubbling fluidized bed reactor using artificial intelligence techniques

Muhammad Faisal Irfan*, Farouq S. Mjalli, Sang Done Kim

*Corresponding author for this work

Research output: Contribution to journalArticle

13 Citations (Scopus)

Abstract

Comparative study of the artificial neural network and mechanistic model was carried out for NO removal in a bubbling fluidized bed reactor. The effects of temperature, superficial gas velocity and ammonia/nitric oxide ratio on the NO removal efficiency were determined and their optimum conditions were estimated by the experimental study, the artificial neural network and mechanistic models as well. The optimum values of ammonia/nitric oxide ratio, temperature and superficial gas velocity for the maximum NO removal efficiency were found to be 1.5, 300 °C and 0.098 m/s, respectively. A mechanistic model was implemented in our previous study [Muhammad F. Irfan, Sang Done Kim and Muhammad R. Usman, 2009] and it was found that this model fitted well only at specific condition i.e. maximum conversion temperature (300 °C). However, it failed to perfectly match with rest of the experimental data points at other temperatures and parametric conditions as well. To improve this, an artificial neural network modeling strategy was applied and its predictions were evaluated which were favorably matched with the experimental data rather than the mechanistic model.

Original languageEnglish
Pages (from-to)245-251
Number of pages7
JournalFuel
Volume93
DOIs
Publication statusPublished - Mar 2012

Keywords

  • ANN
  • Mechanistic model
  • NO removal
  • SCR

ASJC Scopus subject areas

  • Fuel Technology
  • Energy Engineering and Power Technology
  • Chemical Engineering(all)
  • Organic Chemistry

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